Methane (CH4) contributes to about a third of today's anthropogenic global warming. Radiocarbon (14C) measurements of atmospheric CH4 can be used to track its origin: either from biogenic sources (such as agriculture, waste handling, lakes/reservoirs or wetlands) or from fossil sources (e.g. fossil-fuel combustion or leakages from natural gas networks).
Based on a novel CH4 extraction setup, we want to extend the number of atmospheric 14CH4 measurements within the new-starting interdisciplinary SNSF-project RICH, which aims to develop a national radiocarbon inventory of Switzerland for all compartments of the ecosystem.
This work was carried out in the group of Prof. Dr. Sönke Szidat.
References:
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C. Espic, M. Liechti, M. Battaglia, D. Paul, T. Röckmann, S. Szidat;
"Compound-specific radiocarbon analysis of atmospheric methane: a new preconcentration and purification setup"
Radiocarbon, 2019, 61(51), 1461-1476;
doi:10.1017/RDC.2019.76.
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T. Eglinton, H. Graven, S. Szidat, F. Hagedorn;
"Radiocarbon Inventories of Switzerland (RICH): An integrated approach to understand the changing carbon cycle"
Swiss National Science Foundation (SNSF), 2020;
http://p3.snf.ch/project-193770.
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